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New insights into switchable MOF structures

 E-Mail Metal-organic framework compounds (MOFs) consist of inorganic and organic groups and are characterised by a large number of pores into which other molecules can be incorporated. MOFs are therefore interesting for many applications, for example for the storage of gases, but also for substance separation, sensor technology or catalysis. Some of these MOF structures react to different guest molecules by changing their structures. They are thus considered switchable. One of these is DUT-8 , a material that has now been studied at the MX beamlines of BESSY II. MOF crystals can be analysed very well at the MX beamlines, says HZB expert Dr. Manfred Weiss, who heads the MX team. MOF crystals have many things in common with protein crystals. For example, both are interspersed with large pores, which are filled with liquid in the protein crystals, while those in MOFs provide space for guest molecules, Weiss explains.

High-capacity electrodes by valence engineering developed for desalination

 E-Mail Credit: XU Yingsheng Recently, the researchers from Institute of Solid State Physics, Hefei Institutes of Physical Science (HFIPS) of the Chinese Academy of Sciences, by using valence engineering, developed three manganese oxides as electrodes with different Mn valences for high-performance capacitive desalination. Reverse osmosis and thermal distillation are widely used to treat salt water with high salt concentration, but they have disadvantages including high energy consumption and high cost. As an alternative method, capacitive deionization (CDI) technology can remove charged ions from desalt water through electrosorption or pseudocapacitive reaction. However, there are few reports on manganese oxides with lower valence of Mn, compared with the number of reports on MnO2. Hence, whether there is a difference in desalination performance in such different valence states of Mn and the internal reasons are worth exploring.

DNA-based material with tunable properties

 E-Mail IMAGE: On the left, a snapshot of the simulated system a dense solution of supercoiled plasmid. On the right, a more detailed view of the supercoiled fluid showing entanglements between. view more  Credit: © Davide Michieletto, University of Edinburgh and Jan Smrek, University of Vienna While DNA is often idealised as the molecule of life , it is also a highly sophisticated polymer that can be used for next-generation materials. Beyond the fact that it can store information, further fascinating aspects of DNA are its geometric and topological properties, such as knotting and super-coiling. Indeed, very much like a twisted telephone cord, DNA is often found coiled up inside bacteria and other cells and even knotted in viruses. Now, a collaboration of scientists from the Universities of Edinburgh, San Diego and Vienna have started to harness these properties to craft topologically tunable DNA-based complex fluids and soft materials with potential application

Electrons waiting for their turn: New model explains 3D quantum material

 E-Mail IMAGE: The illustration shows electrons in a topological quantum metal waiting to be activated by a magnetic field. Once they start moving, they follow a spiraling helix upwards - in contrast. view more  Credit: Copyright: Jörg Bandmann This new 3D effect can be the foundation for topological quantum phenomena, which are believed to be particularly robust and therefore promising candidates for extremely powerful quantum technologies. These results have just been published in the scientific journal Nature Communications. Dr. Tobias Meng and Dr. Johannes Gooth are early career researchers in the Würzburg-Dresdner Cluster of Excellence ct.qmat that researches topological quantum materials since 2019. They could hardly believe the findings of a recent publication in Nature claiming that electrons in the topological metal zirconium pentatelluride (ZrTe5) move only in two-dimensional planes, despite the fact that the material is three-dimensional. Meng and G

Study of Fe2+ ions contributes to further understanding of magnetoelectric coupling

 E-Mail IMAGE: An example of a scheme of virtual excitations corresponding to the coupling of spins of chromium and iron ions with an electric field. The iron ion, due to the interaction. view more  Credit: Kazan Federal University The authors, Kirill Vasin and Mikhail Eremin, contribute to the theory of electronic and structural properties of FeCr2O4 ferrimagnet. Due to the specific quantum state and the symmetry of FeO4 fragment, it has unusual electric and magnetic properties. Below TOO~150K, it lowers the symmetry with the macroscopic deformations due to the cooperative Jahn-Teller effect. The coupling between macroscopic deformation of the crystal FeCr2O4 and its inner ions shifts was revealed. The team enhanced the microscopic crystal field theory for 3D electrons with Kleiner s correction - the effect of penetrating charges density. It allows to have better prediction of electron-deformation coupling parameters, which is important for magnetostriction application

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