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Sodium-ion batteries (SIBs) are a promising candidate for large-scale energy storage due to the low cost and abundant sodium resources. However, the formation of sodium dendrites on the surface of hard carbon (HC) anodes is the most intractable challenge for full cells during charging, leading to severe performance degradation and safety hazards. Here, a robust additive-induced borate and fluoride-rich interphase is constructed by introducing sodium difluoro(oxalato)borate (NaDFOB) as additive in the ether-based electrolyte to relieve the performance deterioration for SIBs. NaDFOB can particip...

Organic materials have attracted much attention in sodium ion batteries (SIBs) because of their advantages such as being environmentally benign and having high designability. Capacities and cycle life of organic materials are the most important parameters in most research which has been paid much effort to obtain an impressive electrochemical performance on the material level, and the sodium-detachable ability of these materials to directly match with the sodium-free anode is neglected. In this work, one organic sodium salt (C6H2Na2O6) exhibits the unique ability (charging first in half cell) ...

Abstract Hard carbon (HC) is recognized as a promising anode material with outstanding electrochemical performance for alkali metal-ion batteries including lithium-ion batteries (LIBs), as well as their analogs sodium-ion batteries (SIBs) and potassium-ion batteries (PIBs). Herein, a comprehensive review of the recent research is presented to interpret the challenges and opportunities for the applications of HC anodes. The ion storage mechanisms, materials design, and electrolyte optimizations for alkali metal-ion batteries are illustrated in-depth. HC is particularly promising as an anode ma...