"Surface coating engineering of Li-excess cathode additive of lithium-i" by Hyo Bin Lee, Yun Seong Byeon et al.
Silicon based anodes are known to have a high specific capacity and low operating voltage (less than 0.5 V vs. Li/Li+). Even so, the solid electrolyte interphase (SEI) formation induces the severe capacity loss at the first cycle, known as a critical factor in reducing the energy density of lithium-ion batteries (LIBs). To improve the energy density by compensating the initial Li+ loss, the utilization of Li-excess cathode additives has been considered as the most practical strategy for supplying surplus Li+ during the initial charge. Li2NiO2 is an ideal cathode additive thanks to its large ch...